Nonadiabatic transition: concepts, basic theories and applications
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Hence, the notion of isolated potential energy surface may lose the sense. This is what Dr. Takatsuka calls "chemistry without potential energy surfaces". Even in such highly quasi-degenerate electronic states, one can track those complicated nonadiabatic dynamics with the so-called "on-the-fly" method along non-Born-Oppenheimer paths.
In this way, he has studied in depth chemical dynamics and the reaction fields those densely quasi-degenerate states can offer. He is also interested in the laser-control of them. Takatsuka and his coworkers have developed theoretical methodologies to monitor the real-time dynamics of chemical reactions by means of femto-second angle- and energy-resolved pump-probe photoelectron spectroscopy. In particular, he has shown that this method can be applied to the direct observation of nuclear wave packet bifurcation, which takes place as the molecular states pass across avoided crossings or conical intersections.
This prediction has been experimentally confirmed some years later. For instance, Dr. Takatsuka has shown ways to shift the location of conical intersection and to control the associated nonadiabatic passage through it. Another important work by Dr. A continuous wave laser applied to this nonadiabatic system should cause accelerated motions of electrons or dipole moments within the molecule, leading to emission of photons, the frequencies and intensities of which turn out to be very characteristic.
- Nonadiabatic - definition of nonadiabatic by The Free Dictionary.
The emitted lights can be used as finger-prints of molecules and also new optical sources followed by high harmonic generation. These systems can be regarded as nonlinear driven oscillators, which may undergo limit cycle, frequency-locking, chaos, and so on, and will also shed a new light on "quantum nonlinear dynamics". Takatsuka has established, with Prof. McKoy, a stationary-state quantum scattering theory for electron collision by polyatomic molecules within the fixed nuclear approximation, with which ab initio calculations of differential cross sections not only of elastic scattering but also by polarization, Feshbach resonance, electronic-state excitation, and so on, came to become possible.
These scattering phenomena are quite ubiquitous not only in the natural phenomena such as molecular evolution in cosmic space but also even in industrial applications such as those using plasma processes. This theory by Dr. Takatsuka has played a critical role to make a drastic progress in the field of electron collision phenomena. Takatsuka and his led group have made very fundamental contributions to the theoretical frameworks of molecular science. Springer-Verlag Berlin Heidelberg Their download nonadiabatic transition: concepts, basic theories, everyone and record is political blinkers for underlying original and human men.
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